DETERMINATION OF CURRENT AND HISTORIC LOADS OF ATMOSPHERIC DEPOSITION IN THE CZECH REPUBLIC USING ANALYSES OF MOSS AND FOREST FLOOR HUMUS

 

Julie Sucharová, Ivan Suchara* (*Research Institute of Ornamental Gardening, CZ 252 43 Průhonice, Czech Republic; suchara@vuoz.cz)

 

Abstract

            The concentration of fourteen elements (Al, As, Cd. Co, Cr, Cu, Fe, Hg, Mo, Ni, Pb, S, V, Zn) was measured in moss and forest floor humus samples to determine the current and historic large-scale atmospheric loads in the Czech Republic. Multielement analyses of moss and humus provide a credible, quick and relatively cheap means of identifying the relative and absolute actual loads and the relative historic atmospheric loads in large territories. In order to test the biomonitoring techniques on a fine scale, moss and humus matrices were taken in a dense grid of sampling points near the city of Příbram - a multielemental source of pollution. The impacts of mining and smelting polymetallic ores, recycling Pb wastes and mining uranium ore were reliably determined, and historic and current contaminations of 36 elements in hot spots were located in the investigated landscape segment. The obtained results justify us in recommending moss and humus biomonitoring for wider use.

 

Introduction

Large-scale measuring of atmospheric deposition levels at stations is a time-consuming and expensive activity. Analyses of elements in widely used natural matrices may provide an alternative way, as the element content in them correlates significantly with the local atmospheric deposition level. We decided to use analyses of moss and forest floor humus, for large-scale biomonitoring of current and historic atmospheric loads throughout the Czech Republic (50˚N; 15˚E, abbreviated ´the CZ´ in the following text) and for a fine-scale biomonitoring in a landscape segment near a local multielement pollution source.

 

a) Mosses – bioindicators of current atmospheric deposition loads

            Mosses do not have genuine roots and the inflow of water and elements from the ground substrate is slow enough to be negligible, mainly in a group of terrestrial so-called ´feather mosses´. The surface of the above-ground parts of these mosses adsorbs crucial if not entire amounts of nutrients from atmospheric deposition. No wonder that the content of elements in mosses correlates significantly with the current atmospheric deposition levels in a given area (Rühling and Tyler 1970, 1971). It is even easy to calculate the absolute atmospheric deposition levels of elements at a given place from the concentration of elements in moss samples, moss production data and coefficients of element uptake

b) Forest floor humus – an indicator of historic loads

Analyses of individual layers of known age cored from peat bogs, glacials or tills have been used for determination of historic levels of element deposition (e.g., Steinnes 1997, Weiss et al. 1997). Unfortunately, these materials are not distributed in sufficient abundance for large-scale monitoring or screening in central Europe. To solve this problem, we tested forest floor humus of coniferous forests as an alternative matrix with a long memory. Exclusively the H horizon of forest floor was used due to its microbiological resistance. The organic H and deeper soil A horizon are mixed through natural or man-made processes. Hence selective digestion of organic matter in humus samples was needed to eliminate geogenic influence and to determine the retrospective atmospheric deposition loads.

 

Methodology

a) Moss monitoring

            Moss monitoring was carried out in the CZ (78,864 km2) in 1991 and 1995 in the framework of the European moss monitoring programmes (Rühling 1994, Rühling and Steinnes 1998). In the latter monitoring programme, 196 moss samples were taken in a grid of sampling points of 20x20 km and the methods used followed the instructions of the international programmes. Preferably Pleurozium schreberi moss was taken. The concentration of 14 elements (Al, As, Cd, Co, Cr, Cu, Fe, Hg, Mo, Ni, Pb, S, V, Zn) in two-year-old moss segments (1994-1995) was measured by means of the ICP-OES technique. Standard reference materials, moss laboratory standards and recovery tests were used to check the digestion and analytical processes.

b) Humus monitoring

            In contrast to moss monitoring, there was no available standardised method for taking and analysing forest floor humus for large scale monitoring. A technique for sampling and analysing forest floor humus was therefore developed and tested in the CZ in 1993-1995. Retrospective historic loads of the 14 elements were determined throughout the CZ. About 200 samples of humic substances exclusively from H horizons were taken in mull or moder forest floors of Scots pine (Pinus sylvestris), Norway spruce (Picea abies) or mixed forest stands, usually 60-90 years old, in 1995. The mineral (´ash´) content was controlled through the loss-on-ignition technique and its content exceeding of 30% was avoided in taken samples. Concentrations of 14 elements (see moss monitoring above) in organic matter were measured in samples digested through HNO3 + H2O2 using an ICP-OES instrument after centrifugation off undissolved Si and Si-gel. Concentrations of elements were related to the so-called ash-free samples. For more details see Sucharová and Suchara 1998c.

c) Fine-scale monitoring

            The city of Příbram (49˚41´N; 14˚ 00´E), situated in a wooded landscape, was chosen as a model of a multiple source of current and historic air pollution. Polymetallic Ag, Pb, Zn ores with many minority elements were extracted near the city and processed in a local smelting works as recently as the 1970s. Now the smelter located close to the abandoned mine recycles Pb wastes and metals from electronic components. From 1949-1992 uranium ore (uraninite) was extracted from pits on the opposite side of the city.

            In 1999, samples of coniferous forest floor humus and moss (Pleurozium schreberi) were taken along linear transects 15 km in length running radially from the smelter chimney. The transects were 30º apart, and the distance between the sampling points at the transects was 2000 m. Analyses of 36 elements (see Table 2) were carried out by means of the ICP-MS technique. The distribution of current and historic loads of these elements was determined in classed post maps and isoline maps.

 

Results

a) Large-scale moss monitoring

Selected  characteristics of a set of analysed moss samples from the CZ are shown in Table 1. Moss analyses showed very high current atmospheric deposition loads of Al, As, Co, Cr, Hg, Mo, Ni, S, V and Zn in the lignite basin and its surroundings in the northwestern part of the CZ. The chemical industry and power plants are concentrated in this basin. This area is the Czech part of a heavily polluted area known as the ´Black Triangle´. Very high deposition of the above elements and Cd, Cu and Pb were found in the mountains on the northern border of the CZ. Pollutants are transported to this area from distant sources located in the Black Triangle. Very high current deposition levels of Cd, Fe, Mo, Pb, S, and Zn were found in the black coal basins in the northeastern part of the CZ, where coal processing, metallurgical engineering and chemical industries are concentrated. 6.8%, 13.0%, 43.7% and 36.5%, respectively, of the CZ territory suffered from very high, high, moderate and small general atmospheric deposition loads weighted through the concentration of all 14 elements in the moss samples. Analyses of samples taken at identical places in 1991 and 1995 demonstrated a significant decrease in all measured element deposition by between 16% (Cd) and 77% (As), due to the enormous decrease in industrial production and the introduction of a desulphurization programme for the power plants in the CZ in the 1990s. The average concentrations of the elements in the moss samples were very close to the average data published for Germany and Poland. Slightly lower concentrations (about -20%) were found in Austria, but higher concentrations in Slovakia. Colour maps of the distribution of current atmospheric deposition loads, and results with a commentary, can be found in the latest Czech moss monitoring surveys (Sucharová and Suchara 1998a, 1998b).

 

Ele-

ment

Moss

Humus

Min.

Max.

Mean

S.D.

Median

Min.

Max

Mean

S.D.

Mediam

Al

246

1633

625

269.855

548.093

3575

30075

9120

4168

8124

As

0.150

2.796

0.648

0.469

0.503

5.49

167.0

23.8

17.79

19.20

Cd

0.148

2.627

0.392

0.323

0.315

0.328

5.82

0.865

0.559

0.708

Co

0.147

1.876

0.463

0.256

0.390

1.45

17.5

5.15

2.69

4.41

Cr

0.586

59.337

1.937

2.135

1.386

7.48

94.5

26.5

13.28

23.40

Cu

3.452

18.484

7.580

2.272

7.178

8.37

214

29.6

19.13

25.30

Fe

135

5904

531

574.3

400

3043

36998

10874

5.738

9019

Hg

0.029

0.177

0.072

0.027

0.064

0.329

2.26

0.676

0.205

0.656

Mo

0.054

0.944

0.179

0.125

0.143

0.665

7.97

1.97

1.079

1.750

Ni

0.825

15.634

2.354

1.474

1.944

6.26

52.6

18.8

8.11

17.20

Pb

4.144

173.644

15.357

18.402

11.028

52.1

4872

185

348.4

141.00

S

1048

2628

1594

313.5

1554

2259

4747

3045

417

2955

V

0.580

7.844

2.427

1.394

2.001

9.86

125

37.5

19.30

33.20

Zn

24.528

519.511

56.003

56.944

41.871

42.1

446

89.1

42.7

79.3

 

Table 1 Statistics for a set of element concentrations (μg/g) in moss (n=192) and forest floor humus samples (n=192) taken in the CZ in 1995.

 

b) Large-scale humus monitoring

Basic statistics for humus analyses can be found in Table 1. Humus analyses showed that the distribution of historic (humus) and current (moss) loads had similar patterns in the CZ. The reason for this is that industrial centres grew up at certain sites in the second half of the 19th century, and industrial production has continued mainly in these regions in the territory of the present-day CZ. Very high levels of old contaminations were found for Cd, Co, Fe, Hg, Mo, Ni, Pb, V and Zn mainly around the historic centres of the metallurgical and engineering industries in Central Bohemian region. In the industrial lignite basin in the northwestern cross-border area, very high historic loads of Al, As, Co, Cr, Cu, Fe, Mo, Ni, S, and V were found. Large hot spots of high historic contaminations of Cd, Cr, Cu, Fe, Mo, Pb, and Zn were identified in the industrial region surrounding the black coal mines in the northeastern part of the CZ. Generalised data showed that, respectively, very high, high, moderate and low historic deposition loads related to all partial deposition loads of individual elements were found, respectively, in 18%, 24% 30% and 28% of the CZ territory. Relatively small atmospheric deposition loads have generally affected the southern half of the CZ. Detailed interpretation of large scale humus monitoring in the CZ was presented in the CZ national humus survey (Sucharová and Suchara 1998c, Suchara and Sucharová 1999).

c) Fine-scale monitoring of current and historic loads

Table 2 gives information about the range of the absolute current (1998) atmospheric loads of the elements for the city of Příbram and its surroundings determined by moss analyses. ´Typical values´ of deposition are related to the average loads affecting the main of the investigated landscape segment.

The results of principal component analysis showed four factors that may explain more than 70% of the individual element distribution in the analysed matrices. The following factors (pollution sources) were easily identified: the smelter works (chimney, slag piles and the area of the former polymetallic mine) for Ag, As, Bi, Cd, Cu, Fe, Hg, In, Ni, Pb, S, Sb, Se, Tl, Zn (old loads) and Ag, As, Cd, Cu, In, Ni, Pb, Sb, Se, Zn (current loads), former uranium mines for Al, Be, Cr, Cs, Ga, Li, Mn, Rb, Sc, Sr, Th, U, V (old loads) and Al, Be, Ce, Cr, Fe, Ga, La, Li, Nd, Pr, Sc, Th, U, V, Y (current loads), the heat-resistant steel foundry situated 15 km from the city of Příbram for Mo, and geogenic or anthropogenic factors for Tl, Ce, Co, La, Nd, Pr, and V patterns. Complete analytical and graphical results of fine-scale monitoring around the city of Příbram have been presented in a research report (Sucharová and Suchara 1999).

 

 

Ag

Al

As

Bi

Cd

Ce

Uptake coef.

1.10

0.45

0.39

(0.77)

0.72

0.46

Min.-Max.

3.75-124.31

70807-223027

109.2-1409.1

3.07-14.74

41.21-1067.83

100.96-333.72

Typical

4.7-7.0

143333-157667

132.3-198.5

8.4-9.2

107.5-125.4

182.3-196.3

 

Co

Cr

Cu

Fe

Ga

La

Uptake coef.

0.45

0.60

0.46 (0.35-0.57)

0.60

0.49

0.49

Min.-Max.

45.87-286.67

120.4-365.5

3870-308478

43860-143835

29.22-95.04

43.18-152.96

Typical

86.0-114.7

215.0-279.5

7010-9815

86000-107500

47.4-52.7

79.0-92.1

 

Li

Mo

Ni

Pb

S

Sb

Uptake coef.

0.42

0.53

0.46

1.00

0.39

(1.05)

Min.-Max.

46.07-137.91

23.85-258.0

269.22-1318.04

869.5-127452.0

317208-539154

18.43-2899.43

Typical

76.8-92.1

36.5-48.7

420,7-701.1

1935-2580

396923-463077

18.4-36.9

 

Th

U

V

Y

Zn

*Ba, Be, Cs, Hg

In, Mn, Nd, Pr, Rb, Sc, Se, Sr, Tl.

Uptake coef.

0.43

0.865

0.59

0.48

0.85

Min.-Max.

6.0-39.6

3.58-71.88

218.64-1051.68

23.92-86.00

4598-36727

Typical

21-27

6.0-7.5

328-437

37.6-48.4

7588-9106

*For Ba, Be, Cs, Hg, In, Mn, Nd, Pr, Rb, Sc, Se, Sr and Tl the uptake coefficients were not reliably known.

 

Table 2 Absolute minimum, maximum and typical values of atmospheric deposition loads (μg/m2/year) in the city of Příbram and its surroundings assessed from moss analyses and uptake coefficients used.

 

 

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Rühling Å, Steinnes E, Editors (1998), Atmospheric heavy metal deposition in Europe 1995-1996. Nord, 1998, 15.

Rühling Å, Tyler G (1970), Oikos 21: 92-97.

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Suchara I, Sucharová J (1999), In: Proc. from the IVth Intl. Conf. Soil Monitoring. Central Inst. for Supervising and Testing in Agriculture, Brno, pp. 75-78.

Sucharová J, Suchara I (1998a), Biomonitoring of the atmospheric deposition of metals and sulphur compounds using moss analysis in the Czech Republic. Results of the international biomonitoring programme 1995. Průhonice, Res. Inst. Ornamental Gardening, 183 pp.

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Sucharová J, Suchara I (1999), (Multielemental analyses of moss and humus around the city of Příbram. In Czech). Research. Report VaV/610/3/97, Průhonice, Res. Inst. Ornamental Gardening, 104pp.

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Weiss D, Charman DJ, Grattan JP, Cheburkin AK (1997), Water, Air, Soil Pollut. 100: 343-353.